Other Forensic Disciplines

Forensic Disciplines and Lubricant Analysis

  • Distinguished Speaker Series: Candice Bridge, Ph.D. — Lubricants: Revolutionizing Sexual Assault Investigations (8/26/2025)

  • Scope: Forensic disciplines with a focus on lubricants in sexual assault investigations; historical context, lab methods, data analytics, and real-world implications; also includes related topics in entomology, forensic social work, and explosives for broader forensic science context.


Sexual Assault Investigations: Key Statistics and Lab Practices

  • Sexual assaults in America (high-level trend data):

    • 2010: Nearly 1 in 5 (18.3%) women and 1 in 71 (1.4%) men have reportedly experienced a sexual assault in their lifetime.1

    • 2014 (BJS): 33.6% of rapes and sexual assaults were reported (noting most violence is underreported).2

    • 2017 (BJS): 1.4 per 1000 people were raped or sexually assaulted; 28.2% increase from 2016.

  • Note on DNA: Increased condom use may reduce the likelihood of finding DNA evidence in sexual assault cases.1

  • Sources: [1] Black et al., CDC/NIPC; 2011. [2] Truman & Langton, BJS; 2015. http://www.bjs.gov/content/pub/pdf/cv14.pdf

  • 2012 NIJ Study (Los Angeles County, SAKs):

    • 10,895 SAKs not submitted; 1,948 SAKs randomly selected.

    • 1,320 (68%): DNA was found.

    • 699 (36%): full profiles → CODIS.

    • 347 (18%): positive CODIS hits; 320 (16%) – “Offender” hit.

    • 90 (5%): Already convicted.

    • 147 (8%): Identified Offender.

    • 70 (4%): Unidentified Offender.

    • 13 (0.6%): Undetermined.

    • 27 (1.4%): Case-to-Case Hits (matches a CODIS profile regardless of case).

    • 20 (1%): Identity known.

    • 40% of cases were solved without DNA.

    • Key question: What other evidence is probative?

  • Criminal Justice Outcomes (from NIJ study):

    • No new arrests after the 371 kits were tested.

    • Charges filed on one new case; two persons convicted.

    • A suspect was arrested in nearly 40% of cases without DNA.

    • Implication: DNA testing is not always necessary for a plea or conviction in sexual assault cases.

    • Open question: whether uploading unadjudicated profiles into CODIS could help solve future crimes.

  • Practical/strategic implication: Consideration of additional tools beyond DNA to assist in investigations (e.g., lubricant analysis, other trace evidence).


Evidence Submission and Backlogs

  • Why are SAKs not submitted?

    • Not labeled a “backlog” case; backlogs are defined as cases waiting testing in the crime lab or in the lab >30 days.

    • Survey of 2,000+ law enforcement agencies on submission of forensic evidence.

    • Unsovled case proportions (examples): 18% of unsolved SA cases; 14% of unsolved homicides; 23% of unsolved property crimes.

  • Reasons agencies do not submit evidence (percentages):

    • No suspect identified: 44%

    • Uncertain of usefulness: 30%

    • Suspect adjudicated without testing: 24%

    • Case dismissed: 19%

    • Prosecutor did not request testing: 15%

    • Note: The slide shows a mix of rationales; these figures underscore variability in submission decisions.


Sexual Assault Kits: Contents and Time Frames

  • Sexual Assault Kits (SAKs) contents (typical): paper bags/sheets, clothing, bedding, underwear, comb, documentation forms, evidence collection envelopes, collection instructions, blood collection, nail scraper, cotton swabs (blood, saliva, lubricant, vaginal), urine containers, etc.

  • Evidence collection time frames by sample type:

    • Vaginal: Up to 120 hours=5 days120\text{ hours} = 5\text{ days}

    • Anal: Up to 72 hours=3 days72\text{ hours} = 3\text{ days}

    • Oral: Up to 24 hours=1 day24\text{ hours} = 1\text{ day}

    • Bite marks / Saliva on skin: Up to 96 hours=4 days96\text{ hours} = 4\text{ days}

  • Source: Forensic best practices cited (French, L.; Forensic Magazine, 2017).

  • Note: While the specifics include an NIJ/Forensic Magazine reference, the time frames illustrate the urgency of prompt evidence collection in sexual assault cases.


Lubricant Analysis: History, Components, and Methods

  • Context: Lubricant analysis as a tool in sexual assault investigations; main focus on DNA is complemented by lubricant and related trace evidence.

  • Common lubricant components (examples):

    • Tocopheryl Acetate

    • Nonoxynol-9

    • Methyl-Polydimethylsiloxane (PDMS)

    • Hydroxy-PDMS

    • Polyethylene Glycol (PEG)

    • Octylamine

  • GC examples (complex): distinguishing lubricants via gas chromatography patterns; PDMS-containing products versus others.

  • Historical progression in lubricant analysis:

    • 1981 (Blackledge & Cabiness, US Army Crime Lab, Europe): lubricant evidence in rape/sodomy cases; tested petrolatum-based products for comparison; IR inconclusive; fluorescence similar; GC distinguished differences; same-manufacturer products could have similar GC patterns.

    • GC examples included Vaseline and Pro-Line Conditioner.

  • 1994–1996 developments:

    • Condom components identified in SA cases; FTIR traces of PDMS; microscopy showing cornstarch granules, silica, talc; DCI: PDMS and Nonoxynol-9;

    • Guidelines for trace component analysis from latex condoms (1994);

    • Viscosity discrimination of lubricants (1995);

    • FBI Bulletin on lubricant analysis as a factor in investigations (1996).

  • 2001 onward — key researchers and milestones:

    • Maynard (Australia, 2001) protocol for analyzing condoms and personal lubricants.

    • Campbell (NZ, 2007) identification of PDMS oligomers.

    • 2012 (Gross, Germany) use of DART to analyze silicones.

    • 2012 (Musah, NY, USA) DART to characterize SA lubricants & N-9.

    • 2013 (Bradshaw, UK) multidisciplinary analysis of condom-contaminated fingerprints.

    • 2013 (Tonkin, Australia) effect of environment on persistence of lubricants on skin.

  • Overall take: Lubricants have emerged as an analyzable trace with multiple analytical modalities (IR, FTIR, GC-MS, DART-MS, microscopy) that can contribute to linking a suspect, victim, and scene, especially when common DNA evidence is limited.


Analytic Techniques and Instrumentation in Lubricant Analysis

  • Gas Chromatography–Mass Spectrometry (GC-MS):

    • Traditional GC-MS analysis used to distinguish lubricant samples and to identify solvent/solubilizing components.

  • DART-Mass Spectrometry (DART-MS):

    • Ambient/direct ionization (Penning source).

    • High resolution and accurate mass capabilities; comprehensive analysis from 40–2000 m/z; rapid analysis (~5–10 seconds) with little sample prep.

    • Experimental setup (illustrative): mass spectral data in positive-ion mode; parameters such as heater temp ~350°C; MS range 60–1000 amu; typical voltages for ion optics.

    • Study design: subset of samples representing main lubricant marketing types; analysis included neat liquids, hexane extracts, and extracts at 100–350°C temperatures.

  • FTIR (Fourier-transform infrared spectroscopy):

    • Used to identify functional groups (OH, CH, C=O) in neat and extracted residues; peaks noted at ~3351 cm⁻¹ (OH), ~2916 cm⁻¹ (CH sp³), ~2848 cm⁻¹, ~1638 cm⁻¹ (C=C), etc.

  • LC/GC with targeted fragments for PDMS: analyses focusing on PDMS oligomeric ranges and characteristic fragments.

  • Polarized Light Microscopy: used to analyze cornstarch or other granular components in lubricants.

  • Nomenclature snapshot from spectra:

    • Positive ion species: e.g., Glycerol [M+H]+ at 93.0554 (calc), measured 93.0552.

    • [2M+H–H2O] at 167.0906 (calc) vs 167.0919 (meas).

    • Maltol [M+H]+ at 127.0403 (calc) vs 127.0395 (meas).

    • Negative ion forms: Glycerol [M–H]− at 91.0405 (calc) vs 91.0395 (meas).

    • Furoic acid [M–H]−, Aconitic acid [M–H]−, Citric acid [M–H]− with corresponding calculated vs measured masses.

  • Chemometrics (for spectral data):

    • Reduces subjectivity in spectral inspection (Q vs K comparisons).

    • Techniques: Classical least squares? (CA), Principal Component Analysis (PCA), Linear Discriminant Analysis (LDA).

    • Data preprocessing: mass-calibrated, spectral-averaged, background-subtracted datasets.


Chemometrics and Data Analysis in Lubricant Profiling

  • Purpose: Extract patterns and relationships not visible via visual inspection; enhance discrimination among lubricant types.

  • Methods referenced:

    • CA (Correspondence Analysis) / PCA (Principal Component Analysis) / LDA (Linear Discriminant Analysis).

    • Data basis: mass spectral data from DART-MS, including neat and extracted residues; external test sets used for model validation.

  • Principles illustrated by slides:

    • Cluster analysis and heat maps visualize mass spectral datasets and reveal differences within and between lubricant marketing types.

    • PCA reveals grouping by marketing type, with multiple groups showing distinct clusters; some overlap occurs depending on formulation (water-based, silicone, condoms).

  • Example interpretation:

    • Groupings separated into multiple clusters (e.g., Group 1: glycerol; Group 2: glycerol + lidocaine; Group 3: ethoxydiglycol, triethanolamine, benzocaine; etc.).

    • External test and real samples yield high classification accuracy, supporting the ability to distinguish lubricants by composition.

  • Classification outcomes (illustrative numbers):

    • Silicone-based lubricant model: 97.80% correct classification on the validated dataset; 2 of 62 misclassifications.

    • Real samples testing: 92.22% correct classification; 7 of 90 misclassifications; 2 samples could be undetermined (e.g., water).

    • External test set validation (silicone, water, condom): high accuracy with cross-validation; e.g., 93.0557 mass/score threshold; several class thresholds used to separate marketing types.

  • Practical significance: Multivariate chemometric approaches enable objective categorization of lubricants, aiding investigative leads when traditional DNA evidence is limited.


Cluster Analysis, Heat Maps, and PCA in Lubricant Profiling

  • Heat maps: graphical representations of mass spectral datasets; reveal patterns and structure; show both inter-type and intra-type variation among lubricants.

  • PCA (Principal Component Analysis):

    • Reduces dimensionality to reveal grouping of lubricant samples.

    • Example groupings in slides show many brands (Adam & Eve, Astroglide, Jo H2O, KY Jelly, Wet, etc.) forming clusters across several PCs.

    • Demonstrates separation by marketing type and composition (e.g., water-based vs silicone vs condom-associated products; presence of PDMS, anesthetics, flavor/fragrance components).

  • LDA (Linear Discriminant Analysis):

    • Used in conjunction with PCA-derived PCs and cluster groupings to classify samples.

    • External validation and confusion matrices illustrate predictive performance across 12 lubricant groups.

    • Example: classification results show high accuracy for silicone, water, and condom groups, with some misclassifications in more similar formulations.

  • Main takeaway: Multivariate statistics (PCA, CA, LDA) applied to mass-spectral data enable robust discrimination of lubricant types and components, improving investigative leads in sexual assault cases.


Forensic Entomology: Principles and Applications

  • What is forensic entomology?

    • The study/use of insects and other arthropods that feed on decaying remains to aid legal investigations.

    • Subfields: medicolegal (criminal) and urban (criminal and civil) entomology; also relevant to stored products and environmental effects.

  • Primary objective: Estimate the elapsed time since death (ETSD), also called the post-mortem interval (PMI).

  • Additional applications:

    • Secondary movement of a corpse (or other evidence).

    • Post-mortem tampering.

    • Linking perpetrators to crime scenes via insect evidence.

  • At the crime scene:

    • Collection methods include Berlese funnels, leaf litter sampling, soil sampling, and handling of specimens.

    • Guidelines emphasize careful collection around the body and in the surrounding environment; proper preservatives and transport.

  • Practical notes:

    • Insects aid PMI estimation, which can be pivotal in homicide investigations and corroborating timelines.


Forensic Social Work: Roles and Functions

  • Definition: Forensic social work is the practice of social work that intersects with the law.

  • Settings: Community-based child and family services, healthcare, education, child welfare, mental health, substance abuse, social services, juvenile justice, civil and criminal justice systems.

  • Functions of forensic social workers:

    • Providing consultation, education, or training to criminal/juvenile justice systems, law makers, law enforcement personnel, attorneys, paralegals, and the public.

    • Diagnosis, treatment, and recommendations for criminal/juvenile justice populations; assessing mental status, child interests, incapacities, or ability to testify; serving as an expert witness.

    • Screening, evaluating, or treating law enforcement and other criminal justice personnel; policy and program development; mediation and arbitration; teaching, training, supervising; behavioral science research.

  • Roles/areas of practice:

    • Child abuse and welfare; mediation (divorce/separation); expert witness (competency determinations and abuse); mitigation; victims of crime investigations and advocacy; work with defendants and offenders; juvenile justice; refugees and immigration.


Explosives: Definitions, Types, History, Collection, and Analysis

  • Core definitions:

    • Deflagration: Decomposition at a rate much slower than the sonic velocity; propagation by thermal conduction/radiation; slower than the speed of sound; no atmospheric oxygen required.

    • Detonation: A chemical reaction with high temperature and pressure gradient (shock wave) causing instantaneous initiation; detonation velocities range roughly from 1,500 to 9,000 m/s.

  • Types of explosives:

    • Low explosives: Detonation velocity < 1,000 m/s; examples include black powder (KNO3, charcoal, sulfur); smokeless powders (nitrocellulose; single/double/triple base formulations).

    • High explosives: Primary (high sensitivity, primers) and secondary (insensitive) explosives; categories include nitroaromatics, nitrate esters, nitramines.

  • History of explosives: Key milestones

    • Black powder: Origin in China (10th century); Berthold Schwartz improved BP; mining/blasting era; safety fuses (William Bickford) in 1830s.

    • Nitroglycerin (NG): Discovered by Ascanio Sobrero (1846); Alfred Nobel developed NG-based dynamite (1867) using diatomaceous earth; detonation vs. blasting applications; nitro headaches and fumes concerns.

    • Ammonium nitrate: Used for fertilizers, later blasting agents; ANFO developed (1955); shift toward safer handling.

    • Point-of-use synthesis: Inert or safe compounds mixed at the site to generate explosive compounds; binary systems.

  • Advantages/Disadvantages of explosives handling:

    • Advantages: On-site preparation, controlled sizing, reduced storage danger, appropriate detonation when mixed; detonation at very low temperatures.

    • Disadvantages: Cost, time to mix on-site; handling hazards.

  • Collection and processing of residue after an explosion:

    • Debris collection; device reconstruction important; swabs wetted with acetone or water; microscopic examination; aqueous washes for inorganic oxidizers; organic washes for organics; sample filtration and analysis.

  • Field and laboratory detection methods:

    • Field: Ion mobility spectrometers, mobile GC-MS (sniffer capabilities), X-ray detection.

    • Laboratory: GC-MS, GC-Thermal Energy Analysis (TEA), HPLC-MS, IMS.

  • Notable analytic data:

    • Vapor pressures and deflagration points for select explosives (examples):

    • EDGN: vapor pressure at 100°C = 200 Torr; deflagration temperature $T_d$ = 2582°C (illustrative).

    • NG: vapor pressure at 100°C = 0.39 Torr; $T_d$ = 78.6°C.

    • TNT: vapor pressure at 100°C = 0.069 Torr; $T_d$ = 360°C.

    • PETN: vapor pressure at 100°C = 0.0008 Torr; $T_d$ = 26.9°C.

    • RDX: vapor pressure at 100°C = 0.00016 Torr; $T_d$ = 0.31°C.

    • GC-MS (NICI) approaches used for explosive analysis.

  • Historical/modern case examples (terrorist uses of explosives): Beirut 1983 Embassy bombing; 1983 Marine Barracks bombing; Pan Am 103 (Lockerbie) 1988; World Trade Center 1993; Oklahoma City 1995; Jerusalem 1996 Hamas bus attack; Khobar Towers 1996; US Embassy bombings in East Africa 1998; USS Cole 2000; 9/11 attacks 2001; London Tube 2005; Boston Marathon 2013.


Research, Standards, and Forensic Science Landscape

  • Research in forensic science—definition in slides: systematic investigations and studies to establish new knowledge, create theories/methods, improve existing theories, develop a field, bridge knowledge gaps, apply methods to real problems, etc.

  • National Institute of Standards and Technology (NIST) and OSAC: organizational structure for forensic science research and standards; institutional landscape includes national labs, universities, industry partners (Pfizer, Johns Hopkins, Google, Tesla, etc.).

  • OSAC structure and needs:

    • Subcommittees include Biology, Chemistry (Seized Drugs & Toxicology), Forensic Interest, Forensic Toxicology, Digital Evidence, Firearms & Toolmarks, Footwear & Tire, Forensic Anthropology, Forensic Nursing, Forensic Odontology, Imaging, and more.

    • Example note: Digital Evidence Subcommittee reported no identified needs at that time.

  • Research areas and priorities highlighted for technological development:

    • Development of DNA extraction methods, probabilistic genotyping, SNP panels, software solutions for data analysis, alternative matrices, cannabinoids, trace materials, and more.

    • Emphasis on data analytics in toxicology, environmental effects on persistence of traces, and advanced analytical technologies for trace evidence.

  • NIH/Forensic Science Infrastructure:

    • NIH and national labs (NIST, Los Alamos, Savannah River, Ames) contribute to the broader research ecosystem supporting forensics.

  • Innocence Project and wrongful convictions (context from slides):

    • Statistics cited on wrongful convictions and misapplication of forensic science; racial disparities in exonerations; eyewitness misidentification (cross-racial issues); issues of false confessions and coercive interrogations; police/prosecutorial misconduct; inadequate defense.

    • Emphasis on evaluating forensic science claims and improving standards to reduce wrongful convictions.


Forensic Science in Public Discourse and Education

  • Slide content includes a visualization of the Innocence Project statistics:

    • 64% of Innocence Project clients exonerated or freed are Black and/or Latinx.

    • 63% of cases involved eyewitness misidentification (including cross-racial misidentification).

    • 53% of cases involved misapplication of forensic science.

  • Takeaway: Public-facing forensic science must be contextualized with data on errors and biases; ongoing education and standardization are essential to reduce wrongful outcomes.


Mathematical and Statistical Notes (key figures and formulas)

  • Example masses from DART-MS data (illustrative):

    • Positive ion glycerol: calc mass MextGly+=93.0554M_{ ext{Gly}}^{+} = 93.0554; measured 93.055293.0552.

    • Positive ion adduct: [2M+HH2O]+extwithcalc167.0906,extmeasured167.0919.[2M+H-H_2O]^{+} ext{ with calc } 167.0906, ext{ measured } 167.0919.

    • Negative ion glycerol: calc mass MextGly=91.0405,extmeasured91.0395.M_{ ext{Gly}}^{-} = 91.0405, ext{ measured } 91.0395.

    • Negative ion furoic acid: MextFUA=111.0078,extmeasured111.0082.M_{ ext{FUA}}^{-} = 111.0078, ext{ measured } 111.0082.

  • Classification accuracy examples (silicone-based lubricant model):

    • Overall accuracy: ext{Accuracy} = 0.9780 ext{ (97.80%)}; ext{ misclassifications} = 2/62.

    • Real samples: ext{Accuracy} = 0.9222 ext{ (92.22%)}; ext{ misclassifications} = 7/90; ext{ undetermined} = 2.

    • External test set: accuracies show high discrimination among Silicone, Water-based, and Condom groups.

  • PCA/LDA results (illustrative):

    • LDA used with the first 9 PCs from PCA; external validation with 30% test split; observed high separation among lubricant groups with overall accuracy around the mid-to-high 90s percentile for key categories.

  • Pearson correlation (example):

    • Used to compare low-temperature vs high-temperature DART-MS data; e.g., correlation coefficients indicate better separation at lower temperatures for certain flavors/fragrances.

  • Note: All these numerical values are as reported in the slides and serve to illustrate the magnitude of discrimination achievable with chemometric approaches.


Summary: Practical Implications and Ethical Considerations

  • Lubricant analysis expands the forensic toolkit beyond DNA, offering complementary evidence that can link evidence, scenes, and individuals where DNA is absent or inconclusive.

  • The integration of GC-MS, DART-MS, FTIR, and chemometrics enables objective classification of lubricants and related components, reducing subjectivity in interpretation.

  • Ethically, forensic science must address risks of misclassification, bias, and over-interpretation; routine reporting should clearly state limitations and confidence levels, especially in cases with high societal impact (sexual assault, wrongful convictions).

  • The interdisciplinary scope (entomology, social work, explosives) highlights the breadth of forensic science and the importance of cross-disciplinary collaboration for robust investigations and public safety.


Key References and Data Points (select)

  • Sexual assault prevalence and reporting trends: 2010, 2014, 2017 data; condom use can affect DNA yields.

  • NIJ 2012 Los Angeles County SAK study: sample sizes and CODIS outcomes; 40% of cases solved without DNA.

  • Lubricant analysis milestones: IR, GC, GC-MS, FTIR, DART-MS, microscopy, and PDMS-focused work.

  • DART-MS methodology: positive/negative ion modes; rapid acquisition; minimal prep; broad m/z range.

  • Chemometrics in forensic analysis: PCA, CA, and LDA usage; mass-calibrated, background-subtracted datasets.

  • Explosives: history from black powder to ANFO; field and lab detection methods; vapor pressure/deflagration data; NICI-GC-MS.

  • Forensic science ecosystem: OSAC structure; multidisciplinary research; relevance of accurate interpretation to reduce wrongful convictions.

  • Public discourse: Innocence Project statistics on misidentification, misapplication, and wrongful convictions.


Appendix: Quick Glossary of Terms

  • CODIS: Combined DNA Index System.

  • SAK: Sexual Assault Kit.

  • PDMS: Poly(dimethylsiloxane), a silicone compound common in lubricants.

  • DART-MS: Direct Analysis in Real Time Mass Spectrometry.

  • GC-MS: Gas Chromatography–Mass Spectrometry.

  • FTIR: Fourier-Transform Infrared Spectroscopy.

  • PCA: Principal Component Analysis.

  • LDA: Linear Discriminant Analysis.

  • CA: Correspondence Analysis.

  • PMI: Post-Mortem Interval.

  • ETSD: Estimated Time of Death.

  • NICI: Negative-Ion Chemical Ionization (a mode used in GC-MS).