Chem 2 Rate Law
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Try These On Your Own
A series of calculations regarding rate constants was provided:
Activation Energy Calculation:
Rate constants collected at several temperatures yielded a plot of ln k vs. 1/T with a slope of -1.25 × 10^4 K.
The activation energy (Ea) calculated: 104 kJ/mol.
First Order Rate Constant:
Given rate constants at 25 °C (4.82 × 10^–5 s–1) and at 70 °C (1.41 × 10^–2 s–1).
Calculated rate constant at 90 °C: 0.11 s–1.
Rate Constant Factor Change:
For a reaction with an activation energy of 28.9 kJ/mol, determine change from 115 °C to 230 °C.
It increases by a factor of: 7.75.
Half-Life Calculation:
For reaction A → 2B + C with activation energy 85.6 kJ/mol and a half-life of 17.5 h at 225 °C.
The half-life at 166 °C calculated: 282 h.
Summarizing Collision Model Requirements for a Reaction
Effective collisions are necessary for reactions:
Particles must be properly oriented for effective reactions to occur.
The specific orientation for each reaction may vary.
Sufficient energy must be present to overcome the activation energy barrier.
Absence of meeting these criteria results in no reaction.
Chemical Reactions on the Molecular Level
Collision theory stipulates that the reactants must collide to initiate a reaction:
Simple reactions can proceed in one step (e.g., I– + CH3Br → CH3I + Br–).
More complex reactions (e.g., N2(g) + 3 H2(g) → 2 NH3(g)) often occur in multiple steps due to the improbability of all reactants colliding simultaneously with the correct orientation.
The individual steps contribute to what is known as the reaction mechanism.
Reaction Mechanisms
Mechanisms are composed of a series of elementary reactions:
An elementary reaction cannot be simplified further—direct particle interaction occurs.
Reactions may consist of rearranging or decomposing particles (e.g., NO2 → NO radical + O radical + hn).
Reaction Mechanisms (continued)
Validation of proposed mechanisms requires experimental evidence:
A mechanism can be hypothesized but can never be fully proven.
It can, however, be discarded if it does not align with experimental data.
Requirements for a plausible mechanism:
The sum of individual steps must equal the overall balanced reaction.
The mechanism must align with the experimentally determined rate law.
Elementary Reactions and Molecularity
Molecularity refers to the number of reactant particles involved in an elementary reaction:
Unimolecular: Contains one particle.
Bimolecular: Requires two particles.
Termolecular: Requires three particles (rare).
Determining the Rate Law of an Elementary Reaction
The rate law can be established directly from the stoichiometry of an elementary reaction.
Requirement 1 – Adding Up Reactions
Example: 2 NO(g) + 2 H2(g) → N2(g) + 2 H2O(g)
Proposed mechanism involves intermediate species:
2 NO ⇌ N2O2
N2O2 + H2 → N2O + H2O
N2O + H2 → N2 + H2O
Overall reaction is reconcilable with the mechanism.
Requirement 2 – the Mechanism’s Rate Law
Each elementary step has its own activation energy, rate constant, and associated rate law:
The rate of the entire mechanism is limited by the rate-determining step (slowest step) with the highest activation energy.
The rate law of this step must correspond with the experimentally determined rate law for viability.
Determining the Rate Law from a Mechanism
For the overall reaction H2(g) + 2 IBr(g) → I2(g) + 2 HBr(g), the experimentally derived rate law is:
rate = k [H2][IBr]
Proposed mechanism includes:
Step 1: H2 + IBr → HI + HBr (slow)
Step 2: HI + IBr → I2 + HBr (fast)
The rate-determining step is step 1 matching the determined rate law for relativity.
Mechanisms with a Fast Equilibrium Step
Example reaction: 2 NO(g) + O2(g) → 2 NO2(g)
Step 1: 2 NO ⇌ N2O2 (fast)
Step 2: N2O2 + O2 → 2 NO2 (slow)
The rate-determining step is step 2, but includes the reactive intermediate [N2O2], which complicates the rate law.
Mechanisms with a Fast Equilibrium Step (continued)
Solution to rate law challenge involves substitution using concentration relations from step 1's equilibrium, culminating in a comprehensible overall rate law:
Rearranging yields the overall reaction involving measurable concentrations
Result is: rate = k [NO]^2 [O2].